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Spin-polarized electron transport for the altermagnet CrSb
V.D. Esin, 1 D.Yu. Kazmin, 1 A.V. Timonina, 1 N.N. Kolesnikov, 1 and E.V. Deviatov 1 , 2
arXiv:2607.07334v1 [cond-mat.mes-hall]
8
Jul 2026
1 Institute of Solid State Physics of the Russian Academy of Sciences, Chernogolovka, Moscow District, 2 Academician Ossipyan str., 142432 Russia 2 V.L. Ginzburg Research Centre for High-Temperature Superconductivity and Quantum Materials,
P.N. Lebedev Physical Institute of RAS, Moscow 119991, Russia
P.N. Lebedev Physical Institute of RAS, Moscow 119991, Russia (Dated: July 9, 2026) We experimentally investigate spin-polarized electron transport for the centrosymmetric altermag- net CrSb, which is known to reveal both altermagnetic and topological features. We demonstrate pronounced first-harmonic anomalous and second-harmonic non-linear Hall effects for a single-crystal CrSb flake with ferromagnetic nickel contacts, while both effects can not be seen for the reference samples with non-magnetic gold ones. For the anomalous Hall effect, we demonstrate bow-tie hys- teresis loop in Hall voltage, which is usually ascribed to surface spin textures in magnetic materials. The slope of the Hall curve changes a sign for two orientations of the Hall-bar contact configuration for the same sample, i.e. for the same sign of the charge carriers. We interpret the observed sign inversion and bow-tie hysteresis as the joint effect of the alternating bulk spin splitting and spin- polarized topological surface states in CrSb. The pronounced non-linear Hall effect with hysteresis in magnetic field confirms finite Berry curvature dipole under injection of spin-polarized electrons, i.e. the topological features for the altermagnetic candidate CrSb. PACS numbers: 73.40.Qv 71.30.+h
I. INTRODUCTION
Recently, altermagnetic class of materials has been in-
troduced 1 –3 as antiferromagnets with broken the com-
bined spatial-inversion and time-reversal symmetry 4 . In
this case, the spin-opposite sublattices cannot be related
by translation or inversion 5 ,6 , so the up-polarized sub-
band is obtained by π/2 rotation of the down-polarized
one for the simplest example of the d-wave altermag-
net 7 ,8 . As a result, the zero net magnetization is accom-
panied by alternating spin splitting in the k-space 1 ,5,9 .
For altermagnets, the anomalous Hall effect (AHE) as
a hysteresis loop in Hall resistance has been regarded as
the first experimental demonstration of their non-trivial
spin splitting 1 0–14 . While weak ferromagnetism of anti-
ferromagnets has already been known for materials with
strong spin-orbit coupling 1 5 , the specifics of altermag-
netism is the non-relativistic spin-momentum locking 1 .
Usual spin-orbit induced spin-momentum locking is
well known for topological materials, leading to spin po-
larization of the topological surface states 1 6–19 . In mag-
netic topological semimetals, the anomalous Hall effect is
connected with dissipationless surface transport 1 8 . For
non-magnetic systems, AHE is prohibited in the pres-
ence of time-reversal symmetry, while the non-linear Hall
effect (NLHE) 2 0 is predicted as a transverse second-
harmonic voltage response due to the Berry curvature
dipole in momentum space 2 0–24 . In the simplified pic-
ture 2 0 , the longitudinal current generates the effective
sample magnetization, which leads to the Hall effect even
in zero external magnetic field. Hall voltage is therefore
proportional to the square of the excitation current, so it
can be detected as the second-harmonic V 2ω x y transverse
voltage component. NLHE has been demonstrated for a
wide range of materials 2 5–29 , being the direct manifesta-
tion of finite Berry curvature in topological media 2 0 .
Nowadays, it is a common agreement, that AHE
still requires spin-orbit coupling in altermagnetic mate-
rials 1 1,12,30–32 . For example, ARPES (angular-resolved
photoemission spectroscopy) confirms the altermagnetic
nature of spin-spliting in α-MnTe 3 3 . However, the prin-
ciple origin of finite net magnetization 1 1,12,34,35 in MnTe
is the spin-orbit coupling 3 1,32,36–38 . In contrast, spin-
orbit coupling is negligible for centrosymmetric CrSb,
while ARPES confirms high altermagnetic splitting for
this material 3 9,40 . Moreover, signature of topological sur-
face states 4 1,42 has been shown for CrSb 4 3 , so the room-
temperature altermagnetic candidate CrSb reveals both
altermagnetic and topological features 4 4 .
AHE can not be expected for CrSb either from the
topological surface states due to the time-reversal sym-
metry 1 8 or from the bulk altermagnetic spectrum without
spin-orbit coupling 3 1,32 . Similarly, NLHE is prohibited
for centrosymmetric materials 2 0–24 . However, both AHE
and NLHE becomes more intriguing in spin-injection ex-
periments 4 5 due to the alternating bulk spin splitting 3 9,40
and strong spin polarization of the topological surface
states 4 3,44 .
Here, we experimentally investigate spin-polarized
electron transport for the centrosymmetric altermag-
net CrSb, which is known to reveal both altermagnetic
and topological features. We demonstrate pronounced
anomalous and second-harmonic non-linear Hall effects
for a single-crystal CrSb flake with ferromagnetic nickel
contacts, while both effects can not be seen for the refer-
ence samples with non-magnetic gold ones.
2
group P 6 ′ 3 / m ′ m ′ c: two Cr sublattices with opposite spins
are aligned along the c axis, being connected by C6z - a
six-fold rotation combined with a 1/2 translation along
c 4 6,47 . The N´eel temperature is about 705 K, which might
be convenient for possible applications in spintronics.
(a)
Fig. 1 (b) shows a top-view image of the sample. Since
CrSb is a three-dimensional altermagnet, we have to se-
lect relatively thick (about 1 µm) single-crystal flakes. A
thick flake also ensures sample homogeneity for correct
determination of xx- and xy- voltage responses, however,
the desired experimental geometry can not be defined by
usual mesa etching for thick flakes. Instead, the contact
geometry is formed by Ni leads pattern on the SiO 2 sur-
face, as depicted in the inset to Fig. 1 (b). Ni leads are
obtained by lift-off technique after thermal evaporation
of 100 nm Ni film. As a reference, we use Au leads pat-
tern for the samples without spin polarization of charge
carriers.
(b)
FIG. 1. (Color online) (a) The X-ray powder diffraction pat-
tern (Cu K α radiation), which is obtained for the crushed
CrSb single crystal. The single-phase CrSb is confirmed with
the space group P 6 3 / mmc (No. 194). (b) Optical image of
the sample with a 1 µm thick CrSb flake on the ferromagnetic
Ni leads with scheme of electrical connections for one of two
Hall configurations. The leads pattern is shown in the inset:
100 nm thick, 5 µm separated leads allow to realize the cor-
rect Hall (xy-) configuration for two orientations in respect to
the CrSb flake. The depicted Hall configuration is specially
designed to exclude possible admixture of the thermoelectric
effects for reliable NLHE measurements 2 7 .
The mechanically exfoliated ≈100 µm wide CrSb flake
is transferred onto the metallic leads. After initial single-
shot pressing by another oxidized silicon substrate, the
flake is firmly connected to the leads, see Fig. 1 (b). This
procedure provides high-quality contacts, the obtained
samples are electrically and mechanically stable even in
different cooling cycles, which has been verified before for
a wide range of materials 4 8,49,51–53 . Also, the Ni-CrSb
(or Au-CrSb) contacts are protected from any contam-
ination (also oxygen and moisture) by SiO 2 substrate,
as it has been demonstrated for sensitive materials like
black phosphorus 5 3 .
We investigate transverse (xy-) first- and second-
harmonic voltage responses by standard four-point lock-
in technique 2 7,29 . The ac current is applied between two
current contacts in Fig. 1 (b), while the transverse (Hall)
voltage is measured between the potential ones. The sig-
nal is confirmed to be independent of the ac current fre-
quency within 100 Hz – 10kHz range, which is defined by
the applied filters. The measurement are performed at 30
mK temperature in a dilution refrigerator equipped with
a superconducting solenoid. Magnetic field is directed
normally to the sample plane to investigate the first- and
second-harmonic Hall effects.
FIG. 1. (Color online) (a) The X-ray powder diffraction pat-
tern (Cu K α radiation), which is obtained for the crushed
CrSb single crystal. The single-phase CrSb is confirmed with
the space group P 6 3 / mmc (No. 194). (b) Optical image of
the sample with a 1 µm thick CrSb flake on the ferromagnetic
Ni leads with scheme of electrical connections for one of two
Hall configurations. The leads pattern is shown in the inset:
100 nm thick, 5 µm separated leads allow to realize the cor-
rect Hall (xy-) configuration for two orientations in respect to
the CrSb flake. The depicted Hall configuration is specially
designed to exclude possible admixture of the thermoelectric
effects for reliable NLHE measurements 2 7 .
II. SAMPLES AND TECHNIQUE
CrSb single crystals were synthesized by reaction of
pure Cr (99.996%) and Sb (99.9999%), which were mixed
in the stoichiometric ratio and then heated in an evacu-
ated silica ampule up to 1000 ◦ C with the rate of 15 ◦ C/h
in a gradient-free furnace. The load was held at 1000 ◦ C
for 72 hours and then cooled down slowly (11 ◦ C/h) to
the room temperature. The crystals grown are faceted
single crystals with the space group P 6 3 / mmc (No. 194)
and the stoichiometric composition, as confirmed by X-
ray diffraction analysis, see Fig. 1 (a).
CrSb is of hexagonal structure with the magnetic space
We investigate transverse (xy-) first- and second-
harmonic voltage responses by standard four-point lock-
in technique 2 7,29 . The ac current is applied between two
current contacts in Fig. 1 (b), while the transverse (Hall)
voltage is measured between the potential ones. The sig-
nal is confirmed to be independent of the ac current fre-
quency within 100 Hz – 10kHz range, which is defined by
the applied filters. The measurement are performed at 30
mK temperature in a dilution refrigerator equipped with
a superconducting solenoid. Magnetic field is directed
normally to the sample plane to investigate the first- and
second-harmonic Hall effects.
The leads pattern in the inset to Fig. 1 (b) allows to
realize the correct Hall (xy-) configuration for two differ-
ent Hall bar orientations in respect to the CrSb flake: one
configuration 2 7 is shown in Fig. 1 (b), while the current
line is 90 ◦ rotated for the other one 2 9 . In the contacts
area, the leads are of 10 µm width, they are separated
by 5 µm distance, so the voltage probe separation is 20-
80 µm for two different Hall configurations. The correct
choice of the potential contacts is important for AHE and
NLHE measurements. In particular, the contacts config-
uration from Fig. 1 (b) is specially designed for reliable
NLHE measurements, it has been verified to exclude pos-
sible admixture of the thermoelectric effects, see Ref. 2 7
for details.
Table 1 · 11 columns × 0 rows · p.3–3 · CSV
I ac = 2 µA
-0.4 -0.2
I a c = 2 µA
-10
0.0 B (T)
0.2 0.4 -0.4 -0.2 0.0 0.2 0.4
B (T)
FIG. 2. (Color online) Anomalous Hall effect for the CrSb
sample with ferromagnetic Ni contacts. (a) AHE hysteresis is
depicted as the magnetic field dependence of the transverse
voltage V 1ω x y for two field sweep directions for the contacts
configuration from Fig. 1 (b). Inset shows V 1ω x y (B) curves for
the reference sample with normal gold contacts, no AHE can
be seen in this case. (b) V 1ω x y (B) hysteresis for another Hall
configuration, which is 90 ◦ rotated in respect to the one in
(a). The AHE slope is inverted in this case for the same CrSb
flake and for the same magnetic field orientation. For both
Hall configurations, V 1ω x y (B) curves strongly resemble bow-
tie magnetization hysteresis loops 5 5,56 , which is confirmed in
the inset for another sample. The data are obtained at T =
30 mK temperature for the ac current amplitude I a c = 2µA.
III. EXPERIMENTAL RESULTS
Fig. 2 (a) shows typical AHE signal as the magnetic
field dependence of the transverse voltage V 1ω x y for the
sample with ferromagnetic Ni contacts. The data are
obtained for the contacts configuration from Fig. 1 (b)
at T = 30 mK temperature. The ac current amplitude
I a c = 2µA guarantees the linear regime, e.g. it do not
lead to the sample overheating for the low characteristic
longitudinal (xx-) sample resistance ≈ 0.5Ω. The maxi-
mum Hall resistance is 5 mΩ in Fig. 2 (a), it corresponds
to Hall resistivity 0.5 µΩ·cm for 1 µm thick CrSb flake,
which is at least one order of magnitude smaller than the
usual values in magnetic materials 1 1,12,54 . To improve
the signal to noise ratio for low V 1ω x y (B) values, we use
multiple curves averaging, so the hysteresis in V 1ω x y (B)
can be clearly seen for two magnetic field sweep direc-
tions in Fig. 2 (a).
This result is quite unusual for CrSb, since no AHE can
be expected without spin-orbit coupling in altermagnetic
materials 3 1,32,36,37 . We also do not observe any notice-
able AHE signal for the reference samples with normal
gold contacts, as depicted in the inset to Fig. 2 (a), so
the observation of AHE should be a consequence of the
spin-polarized current injection from the ferromagnetic
Ni contacts.
The leads pattern in the inset to Fig. 1 allows to re-
alize another Hall (xy-) contact configuration, where the
0.0
0.1 0.2 0.3 0.4 0.5
I (mA)
FIG. 3. (Color online) Non-linear Hall effect 2 5–29 for the ferro-
magnetic Ni contacts as a quadratic second-harmonic Hall-like
response V 2ω x y ∼ I 2 to ac excitation current I. The curves are
depicted for two 30 mK and 1.2 K temperatures as blue and
red ones, respectively. V 2ω x y ∼ I 2 law is confirmed in the inset
as strictly linear V 2ω x y (I 2 ) dependence for high ac excitation
values. The second-harmonic Hall voltage V 2ω x y is one order of
magnitude smaller for the reference sample with Au contacts
for the same contact configuration, as depicted by the black
curve. The data are obtained in zero magnetic field.
current line is 90 ◦ rotated in respect to the previous case,
the result is depicted in Fig. 2 (b). The V 1ω x y (B) hystere-
sis is of the same ±0.3 T width in Fig. 2 (b), but of lower
amplitude in comparison with one in Fig. 2 (a), the lat-
ter can be ascribed to geometrical factor. However, the
slope changes a sign in Fig. 2 (b), which can not be ex-
pected for the same flake and the same magnetic field
orientation 1 3,14,54 : in normal magnetic field, the angle
between the magnetic field and the current is the same
for two Hall bar configurations in Fig. 2. Since the slope
of the V 1ω x y (B) Hall curve is determined by the sign of the
charge carriers and the magnetic field direction, it should
not depend on the current line orientation in respect to
the CrSb flake.
Also, the hysteresis loops strongly resemble a bow-
tie magnetization hysteresis loop 5 5,56 in Fig. 2: the dis-
tance between the curves for opposite sweep directions is
smaller at zero field/zero voltage, which can be even bet-
ter seen for another sample in the inset to Fig. 2 (b). The
bow-tie hysteresis in magnetization is usually ascribed to
surface spin textures in magnetic materials 5 5,56 .
Fig. 3 shows the effect of spin-polarized current on the
NLHE, i.e. on the second harmonic of the transverse
(Hall) voltage V 2ω x y . For the CrSb sample with ferro-
magnetic Ni contacts, typical behavior of the non-linear
Hall effect 2 5–29 is demonstrated as a quadratic transverse
Hall-like response V 2ω x y ∼ I 2 to ac excitation current I.
In contrast, the second-harmonic Hall voltage is one or-
der of magnitude smaller for the reference sample with
Au contacts in Fig. 3, the data are obtained for the same
contact configuration. For NLHE measurements, we only
use the contact configuration depicted in Fig. 1 (b), to
4
0.1 0.2 0.3 0.4 0.5
0
2
4
B = 0 T
V 2 ω xx
(a)
V
2
ω
x
y
(
µ
V
)
I (mA) -0.4 -0.2 0.0 0.2 0.4
4.76
4.80
4.84 (b)
V
2
ω
x
y
(
µ
V
)
B (T)
I a c = 0.5 mA
-0.4 -0.2 0.0 0.2 0.4
0.02
0.03
V
2
ω
x
y
(
µ
V
)
B (T)
FIG. 4. (Color online) (a) Non-linear Hall effect for another
sample with ferromagnetic Ni contacts in zero magnetic field.
The magenta curve shows the longitudinal second-harmonic
voltage V 2ω x x , which is one order of magnitude smaller. (b)
Hysteresis in V 2ω x y for two magnetic field sweep directions at
I a c = 0.5 mA for spin-polarized transport. Inset shows no
V 2ω x y (B) field dependence for the reference sample with gold
contacts. The data are obtained at T = 30 mK temperature.
reliably exclude the thermoelectric effects, as it has been
demonstrated in Ref. 2 7 .
For NLHE, wide current interval is important to ob-
serve non-linear effects. The NHLE curves V 2ω x y (I) still
depend on temperature in 30 mK–1.2 K range, see red
and blue curves, so the ac excitation do not overheat the
sample. Moreover, sample overheating would lead to di-
minishing of the measured voltage, while the V 2ω x y ∼ I 2
dependence is well confirmed for high ac excitations in
the inset to Fig. 3.
Qualitatively similar ∼ I 2 NLHE dependence is repro-
duced for another sample with ferromagnetic Ni contacts,
see Fig. 4 (a). The longitudinal second-harmonic voltage
V 2ω x x is negligible in comparison with the Hall V 2ω x y one,
which confirms well-defined experimental geometry and
high sample homogeneity.
As well as the first harmonic in Fig. 2, the second-
harmonic Hall voltage shows hysteresis for two magnetic
field sweep directions, see Fig. 4 (b). The hysteresis loops
are of similar widths in Figs. 2 and. 4 (b). In contrast,
there is no V 2ω x y (B) field dependence for the reference
sample with gold contacts, as it is shown in the inset to
Fig. 4 (b).
We should conclude, that for the altermagnet CrSb
both the first-harmonic anomalous and the second-
harmonic non-linear Hall effects can only be observable
for spin-polarized charge carriers.
IV. DISCUSSION
Both AHE and NLHE can not be expected for non-
magnetic and centrosymmetric CrSb, which we confirm
for the reference CrSb samples with gold contacts in
Figs. 2,3,4. Also, the stoichiometric CrSb composition
was verified by X-ray diffraction analysis, see Fig. 1 (a),
so one can be sure in quality of our CrSb material. More-
over, the AHE slope inversion in Fig. 2 can not be ex-
pected even in magnetic materials for the same flake (i.e.
for the same sign of the charge carriers) and the same
magnetic field orientation. Thus, observation of AHE
and NLHE should be connected with spin injection into
the altermagnetic crystal CrSb.
Let us start from the anomalous Hall effect in
Fig. 2. In principle, CrSb exhibits low magnetocrys-
talline anisotropy energy, enabling the manipulation of
the N´eel vector in CrSb films through a suitable ferro-
magnetic substrate, so the anomalous Hall and Nernst
conductivities appear for the canted N´eel vector 5 7 . How-
ever, this effect can only be observable within the bulk
spin-relaxation length, i.e. near the contact regions in
our experiment. Instead, we demonstrate the anomalous
Hall effect for macroscopic (20-80 µm) contact separa-
tion. On the other hand, Weyl topological surface states
were shown for CrSb 4 3,44 . The states with opposite spin
projections are counter-propagating for the vanishing net
magnetization in CrSb, so there is no net AHE for the
current injection from spin-unpolarized gold contacts 1 8 ,
as we corfirm for the reference samples. In contrast,
spin injection from the ferromagnetic Ni contacts leads to
the charge imbalance between counter-propagating sur-
face states and, therefore, to the anomalous Hall effect
in Fig. 2. The effect is observable for macroscopic dis-
tances due to the topological protection of charge trans-
port within Weyl surface states. The hysteresis width in
Fig. 2 should be connected with Ni contact remagnetiza-
tion, i.e., with the change of the spin polarization of the
injected carriers.
However, this picture is only valid for the directions
of full spin compensation in bulk altermagnetic spec-
trum. For other directions, AHE is affected by periodic
bulk altermagnetic magnetization 5 8 , which leads to the
direction-dependent sign of the AHE slope in Fig. 2. In
this case, the bow-tie hysteresis loops in Fig. 2 is the re-
sult of interaction 5 5,56 between the bulk alternating spin
splitting and the surface spin polarization from the topo-
logical surface states 4 3,44 . Thus, the AHE can be ex-
plained as the joint effect of the k-dependent bulk alter-
magnetic spin polarization and spin-polarized topological
surface states for the spin-polarized charge carriers in the
altermagnetic candidate CrSb.
Similar mechanism of spin injection is valid for the non-
linear Hall effect in Figs. 3 and 4. In general, NLHE 2 5–29
arises from the Berry curvature dipole in momentum
space 2 0 . One can not expect non-zero Berry curvature
dipole for centrosymmetric CrSb, which is confirmed by
negligible V 2ω x y for the reference sample with gold contacts
in Fig. 3. However, spin injection leads to the charge im-
balance between the topological surface states, and, in
order, to finite Berry curvature dipole due to the bulk-
5
boundary correspondence, which appears as finite V 2ω x y
transverse voltage in Figs. 3 and 4.
Another possibility to have finite second-harmonic re-
sponse is proposed in Ref. 5 9 . The flow of electric current
in an altermagnet could result in the formation of homo-
geneous electron spin orientation in the sample, which
is quadratic in the current magnitude and does not re-
quire broken inversion symmetry. In principle, the elec-
tron spin orientation could be detected by ferromagnetic
contacts, however, the effect should be observed primary
for the xx- contact configuration. In contrast, the lon-
gitudinal second-harmonic voltage V 2ω x x is negligible in
comparison with the Hall V 2ω x y one in Fig. 4 (a).
The second-order V 2ω x y (B) NLHE response is sensitive
to the external magnetic field 6 0,61 . Being determined by
spin injection from the ferromagnetic Ni contact, NLHE
voltage shows hysteresis within the same field range in
Fig. 4 (b), as the first-harmonic AHE response in Fig. 2.
It is worth mentioning, that there is no field dependence
for the reference sample, as it is shown in the inset to
Fig. 4 (b). Also, NLHE should be affected by the bulk al-
ternating spin splitting 5 8 similarly to AHE, which might
be responsible for very different V 2ω x y values for samples
in Figs. 3 and 4 (a).
V. CONCLUSION
As a conclusion, we experimentally investigate spin-
polarized electron transport for the centrosymmetric al-
termagnet CrSb, which is known to reveal both alter-
magnetic and topological features. We demonstrate pro-
nounced anomalous Hall and second-harmonic non-linear
Hall effects for a thin single-crystal CrSb flake with fer-
romagnetic nickel contacts, while they can not be seen
for the reference samples with non-magnetic gold ones.
For the anomalous Hall effect, we demonstrate bow-tie
hysteresis in Hall voltage, which is usually ascribed to
surface spin textures in magnetic materials. The slope of
the Hall curve changes a sign for two Hall bar orientations
for the same sample, i.e. for the same sign of the charge
carriers. We interpret the observed sign inversion and
bow-tie hysteresis as the joint effect of the k-dependent
bulk altermagnetic spin polarization and spin-polarized
topological surface states for the altermagnetic candidate
CrSb. The pronounced non-linear Hall effect with hys-
teresis in magnetic field confirms finite Berry curvature
dipole under injection of spin-polarized electrons in al-
termagnet CrSb.
ACKNOWLEDGMENTS
We wish to thank S.S Khasanov for X-ray sample
characterization and Vladimir Zyuzin for valuable dis-
cussions. We gratefully acknowledge financial support
by the Russian Science Foundation, project RSF-26-12-
00001, https://rscf.ru/project/26-12-00001/
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